研究方向:
多孔与低维纳米材料;CO2催化转化;人工光合成太阳能燃料催化;环境催化
教育经历:
1998-2003,中国科学院上海硅酸盐研究所,材料科学与工程,博士学位
工作经历:
2003—至今,中国科学院上海硅酸盐研究所,高性能陶瓷和超微结构国家重点实验室,助理研究员、副研究员、研究员
2012.3-8,澳大利亚昆士兰大学,访问学者
曾获得奖励、荣誉称号:
上海市青年科技启明星 (2008)
上海自然科学一等奖 (排名第5,2009)
中科院卢嘉锡青年人才奖 (2010)
中科院青年创新促进会会员 (2012-)
Clarivate高被引科学家 (2018)
负责的科研项目:
[1] 上海市“科技创新行动计划”国际科技合作项目(2020.10-2023.9)“新型人工光合成体系的构建与CO2高效催化转化”,(20520711900)
[2] 国家重点研发计划政府间国际合作重点项目(2019.1-2021.12)“基于二维纳米片的环境催化剂构筑与性能研究”,( 2017YFE0127400)
[3] 国家自然科学基金面上项目(2019.1-2022.12)“低维纳米CeO2表面氧空位的稳定与CO2光催化还原性能的关联机制”,(51872317)
[4] 国家自然科学基金面上项目(2012.1-2015.12)“基于介孔空心球的CO2新型吸附剂的设计制备与性能研究”,(21177137)
[5] 上海市青年科技启明星计划(A类)(2008.7.30-2010.7.31),“新型介孔医用吸附剂的研究”,(08QA1407400)
[6] 国家自然科学基金项目(2008.1-2010.12)“新型可磁分离介孔重金属离子吸附剂的研究”,(50702072)
[7] 中国科学院创新专项基金资助项目(2005.1.1-2007.6.31)“Fe3O4磁性核/介孔SiO2壳复合材料的制备和性能研究”
[8] 上海市纳米专项 (2005.1.1-2006.12.31)子课题“CNT/介孔SiO2复合介观结构材料的制备和性能研究”(0452nm056)
科研工作简介:
围绕太阳能燃料催化合成、CO2催化转化、空气污染物催化净化等目标,设计合成新型多孔与低维纳米材料,研究材料组成-结构-性能间的构效关系,阐明催化过程中的基本反应机制,并开展相关的应用研究。在Angew Chem、Adv Mater、Nano Energy、ACS Catal等期刊发表论文130余篇,H因子56。
1. CO2转化为高价值化学品
设计合成新型的光(电)催化剂,将二氧化碳转化为高附加值化学品。高的产物选择性和高的催化转化效率是我们亟待突破的关键目标。
2. 原子级位点的设计构建及其在催化反应中的作用
发展多种策略,在催化剂中引入原子级位点(单原子、空位缺陷等),优化催化剂的电子结构,调控反应途径,增强催化性能。
3.低浓度空气污染物的催化净化
由于动力学受限,低浓度污染物的去除一直是一个重大挑战。通过构建具有丰富活性位点的光热催化剂材料,在高空速下实现了对低浓度空气污染物的去除。
4. 催化反应机制的原位实时研究
我们搭建了高水平的反应实时原位拉曼-红外-质谱研究平台,可以深入研究材料在真实反应条件下表面物种的变化,推演反应路径,阐明反应机制,由此可以指导催化剂的理性设计。
近3年代表性论文:
[1] Yang Wang, Jinyu Dai, Min Wang, Fenggang Qi, Xixiong Jin, Lingxia Zhang*, Enhanced toluene oxidation by photothermal synergetic catalysis on manganese oxide embedded with Pt single-atoms, Journal of Colloid and Interface Science, 2023, 636, 577-587.
[2] Chengchao Jin*, Jundi Ai, Daiming Liu, Lining Tan, Liang Cao, Binglin Shen, Lingxia Zhang*, Significantly enhanced piezocatalytic activity of BaTiO3 by regulating the quenching process, Journal of Materials Chemistry A, 2023, 11, 10360-10370.
[3] Rongyan Wang, Zhenbin Wang*, Lingxia Zhang*, Qiang Wang, Zhengliang Zhao, Weimin Huang, Jianlin Shi*, Computation-Aided Discovery and Synthesis of 2D PrOBr Photocatalyst, ACS Energy Letters, 2022, 7, 1980-1986.
[4] Xiaoyao Li, Min Wang*, Rongyan Wang, Meng Shen, Ping Wu, Zhengqian Fu, Min Zhu*, Lingxia Zhang*, A distinctive semiconductor-metalloid heterojunction: unique electronic structure and enhanced CO2 photoreduction activity, Journal of Colloid and Interface Science, 2022, 615, 821-830.
[5] Xia Ma, Jianjian Tian, Min Wang, Meng Shen, Lingxia Zhang*, Polymeric carbon nitride supported Bi nanoparticles as highly efficient CO2 reduction electrocatalyst in a wide potential range, Journal of Colloid and Interface Science, 2022, 608, 1676–1684.
[6] Min Wang, meng Shen, Xixiong Jin, Jianjian Tian, Yiran Shao, Lingxia Zhang*, Yongsheng Li, Jianlin Shi*, Exploring the enhancement effects of hetero-metal doping in CeO2 on CO2 photocatalytic reduction performance, Chemical Engineering Journal, 2022, 427, 130987.
[7] Bin Yang, Yifu Wang, Longtai Li, Biao Gao, Lingxia Zhang*, Limin Guo*, Probing the morphological effects of ReOx/CeO2 catalysts on the CO2 hydrogenation reaction, Catalysis Science & Technology, 2022, 12, 1159-1172.
[8] Xixiong Jin, Lingxia Zhang*, Jianlin Shi, Electronic Structure Regulations of Polymeric Carbon Nitride via Molecular Engineering for Enhanced Photocatalytic Activity, Solar RRL, 2021, 2100569.
[9] Xia Ma, Jianjian Tian, Min Wang, Xixiong Jin, Meng Shen, Lingxia Zhang*, Metal-organic frameworks derived carbon supported Cu-In bimetallic nanoparticles for highly selective CO2 electroreduction to CO, Catalysis Science & Technology, 2021, 11, 6096-6102.
[10] Meng Shen, Min Wang, Qiang Wang, Jianjian Tian, Lingxia Zhang*, Lianzhou Wang*, Jianlin Shi*, A Ti-OH bond breaking route for creating oxygen vacancy in titania towards efficient CO2 photoreduction, Chemical Engineering Journal, 2021, 425, 131513.
[11] Qiang Wang, Xia Ma, Ping Wu, Bing Li, Lingxia Zhang*, Jianlin Shi*, CoNiFe-LDHs decorated Ta3N5 nanotube array photoanode for remarkably enhanced photoelectrochemical glycerol conversion coupled with hydrogen generation, Nano Energy, 2021, 89A, 106326.
[12] Meng Shen, Lingxia Zhang*, Jianlin Shi*, Defect Engineering of Photocatalysts towards Elevated CO2 Reduction Performance, ChemSusChem, 2021, DOI: 10.1002/cssc.202100677.
[13] Tian Jianjian, Rongyan Wang, Meng Shen, Xia Ma, Heliang Yao, Zile Hua, Lingxia Zhang*, Bi-Sn oxides for highly selective CO2 electroreduction to formate in a wide potential window, ChemSusChem, 2021, 14(10), 2247-2254.
[14] Qiang Wang, Lingxia Zhang*, Bing Li*, Hongmin Zhu*, Jianlin Shi, 3D interconnected nanoporous Ta3N5 films for photoelectrochemical water splitting: thickness-controlled synthesis and insights into stability, SCIENCE CHINA Materials, 2021, 64(8), 1876-1888.
[15] Jinajian Tian, Min Wang, Meng Shen, Xia Ma, Zile Hua, Lingxia Zhang*, Jianlin Shi, Highly Efficient and Selective CO2 Electro-Reduction to HCOOH on Sn Particle-Decorated Polymeric Carbon Nitride (Very Important Paper), ChemSusChem, 2020, 13, 6442–6448.
[16] Qiang Wang, Lingxia Zhang*, Yangkun Guo, Meng Shen, Min Wang, Bing Li*, Jianlin Shi, Multifunctional 2D porous g-C3N4 nanosheets hybridized with 3D hierarchical TiO2 microflowers for selective dye adsorption, antibiotic degradation and CO2 reduction, Chemical Engineering Journal, 2020, 396, 125347.
[17] Min Wang, Meng Shen, Xixiong Jin, Jianjian Tian, Yajun Zhou, Yiran Shao, Lingxia Zhang*, Yongsheng Li*, Jianlin Shi*, Mild generation of surface oxygen vacancies on CeO2 for improved CO2 photoreduction activity, Nanoscale, 2020, 12, 12374.
[18] Xixiong Jin, Rongyan Wang, Lingxia Zhang*, Rui Si*, Meng Shen, Min Wang, Jianjian Tian, Jianlin Shi*, Electron Configuration Modulation of Nickel Single Atoms for Elevated Photocatalytic Hydrogen Evolution, Angewandte Chemie International Editon, 2020, 59, 6827-6831.
全部发表论文:https://publons.com/researcher/2564908/lingxia-zhang/
课题组信息:https://www.sic.cas.cn/JLShi/